表題番号:2023C-458 日付:2024/02/06
研究課題ペレット状ベントナイトの飽和過程における膨潤圧に及ぼす温度の影響
研究者所属(当時) 資格 氏名
(代表者) 理工学術院 創造理工学部 助教 阮 坤林
研究成果概要

Addressing issues related to high level radioactive waste (HLW) from nuclear power industry is an important task for researchers. Deep geological disposal method, which intends to seal HLW deeply underground, was chosen by many countries to deal with HLW. In a Japanese deep geological disposal project, a multi-barrier system, including vitrified waste, stainless over-pack containers, buffer materials, and host rock, is planned to be constructed more than 300 m underground to prevent the leakage of HLW. As indicated by numerous studies, bentonites and their based materials were selected as candidate buffer materials because of their low permeability. Pelleted bentonite has recently been considered as a candidate buffer material. The purpose of using pelleted bentonite as a buffer material is to avoid the challenges identified in the full-scale mock-up study, such as improved workability during barrier installation. Bentonite pellets can be installed using pneumatic projection techniques, which makes backfilling operations easier and potentially robotic.

In addition to low permeability, another important characteristic of bentonite is its high self-healing ability. As important ingredients for evaluating self-healing capacity, swelling pressures (ps) during saturation, including pressures at peak (ppeak), valley (pvalley), re-peak (pre-peak) and equilibrium (peq) points in swelling curve had been studied by experiments. Among those swelling pressures, most scholars examined peq instead of ppeak, pvalley, and pre-peak. However, experimental conditions strongly affect ppeak, pvalley and pre-peak. Meanwhile, findings from the study of ppeak, pvalley, and pre-peak can elucidate the swelling mechanisms during saturation. Devoting greater attention and making greater effort to assess ppeak, pvalley, and pre-peak are necessary.

In this study, swelling pressure tests were conducted at 25, 50, and 80 °C to elucidate temperature effect on swelling pressures at peak, valley, re-peak and equilibrium points (ppeak, pvalley, pre-peak andpeq) in swelling pressure evolution curve. A pellet bentonite, Kunigel-GX, was used to investigate ppeak, pvalley, pre-peak, and peq at different temperatures. Experimentally obtained results were the followings: 1) ppeak, pvalley, pre-peak, and peq of Kunigel-GX decreased as temperature rises and increased as dry density increases; 2) Kunigel-GX was found to have larger values of (peq-pvalley) at higher dry density and lower temperature conditions.